Laurence Olivier

Priest

Julie Harris

Maria (Priest's Mistress)

George C. Scott

Police Lieutenant

Martin Gabel

Chief of Police

Roddy McDowall

Mestizo

Keenan Wynn

Wine Merchant

Patty Duke

Coral

Val Avery

Leonardo Cimino

Frank Conroy

Padre José

Cyril Cusack

Tench

Roger De Koven

Mildred Dunnock

Spinster

Thomas Gomez

Delgado

Rose Gregorio

Mark Lenard

Joanna Merlin

Mildred Natwick

Tim O'Connor

Florence Stanley

Fritz Weaver

James Coco

Soldier (uncredited)